Chang-Zhu-Tan city cluster has low-carbon “two-oriented” society development advantages of good natural resources and government environment as well as construction experience of low-carbon villages and cities home and abroad. Thus, some serious problems, such as: low economic benefit; unbalanced development between cities and villages; people and land conflict as well as serious environment pollution, bring sever challenge to its low-carbon development. According to its market investigation and data analysis, “two-oriented” villages and cities of Chang-Zhu-Tan city cluster should adhere to developing strategies of ecology priority and low-carbonization for agriculture industrialization.